1990 •
Third-Order Electric Susceptibilities of Halogen-Bridged Mixed-Valence Pt Complexes: [Pt(en)2][Pt(en)2X2](ClO4)4, X=Cl, Br, I, en=ethylenediamine
Authors: Yoshiki Wada, Masahiro Yamashita
Venue: Japanese Journal of Applied Physics
Type: Publication
Abstract: Third-order electric susceptibilities, χ(3) zzzz(-3ω, ω, ω, ω), of the halogen-bridged mixed-valence Pt complexes, [Pt(en)2][Pt(en)2X2](ClO4)4, (X=Cl, Br, I) are calculated using a three level model, taking account of the ground state and odd and even charge-transfer excitons. The values obtained are in the range of 10-12∼10-8 esu and are comparable to, or slightly larger than those observed in polydiacetylenes.
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